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Vortex Stability and Magnetic Disorder Tolerance in Magnetic High-Entropy Alloy Superconductor NbTaTiZrNi

  • Rahmatul Hidayati
  • , Jin Hee Kim
  • , Jae Hyun Yun
  • , Kwan Young Lee
  • , Dilanath Adhikari
  • , Heon Jung Kim
  • , Beongki Cho
  • , Jong Soo Rhyee*
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

2 Scopus citations

Abstract

High-entropy alloy (HEA) superconductors offer mechanical robustness and tunable compositions. We report the synthesis and characterization of a Ni-containing HEA, NbTaTiZrNi, which exhibits superconductivity with Tc ≈ 7.1 K and weak itinerant ferromagnetism up to 300 K, with coercive fields Hcoer ≈ 100–300 Oe. While magnetic elements often suppress superconductivity via pair breaking, Tc in this Ni-containing alloy remains comparable to nonmagnetic Ta1/6Nb2/6Ti1/6Zr1/6Hf1/6 (Tc ≈ 7.8 K). Thermomagnetic flux avalanches are not observed, and critical current densities reach 104–105 A cm–2 at 2 K, indicating robust vortex stability in this composition. Electrical resistivity, magnetization, and specific-heat measurements indicate conventional s-wave superconductivity with intermediate electron–phonon coupling (λ ≈ 0.7). The observed vortex-pinning behavior is consistent with a mixed landscape of grain-boundary and point-like defects, likely influenced by configurational disorder and Ni distribution, though Fe-rich secondary phases may also contribute. These results demonstrate that this specific Ni-containing HEA exhibits robust superconductivity with flux-stable behavior, providing a platform for further exploration of high-performance superconductors in cryogenic applications.

Original languageEnglish
Pages (from-to)3482-3496
Number of pages15
JournalACS Applied Electronic Materials
Volume8
Issue number8
DOIs
StatePublished - 28 Apr 2026

Bibliographical note

Publisher Copyright:
© 2026 American Chemical Society

Keywords

  • High-entropy alloy (HEA)
  • Magnetic elements
  • Magneto-thermal stability
  • Superconductivity
  • Vortex avalanches

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Materials Chemistry
  • Electrochemistry

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