Sequential Deposition of CH3NH3PbI3 on Planar NiO Film for Efficient Planar Perovskite Solar Cells

Long Hu; Jun Peng; Weiwei Wang; Zhe Xia; Jianyu Yuan; Jialing Lu; Xiaodong Huang; Wanli Ma; Huaibing Song; Wei Chen; Yi Bing Cheng; Jiang Tang

doi:10.1021/ph5000067

Sequential Deposition of CH₃NH₃PbI₃ on Planar NiO Film for Efficient Planar Perovskite Solar Cells

Long Hu
, Jun Peng
, Weiwei Wang
, Zhe Xia
, Jianyu Yuan
, Jialing Lu
, Xiaodong Huang
, Wanli Ma^*
, Huaibing Song
, Wei Chen
, Yi Bing Cheng
, Jiang Tang

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

266 Scopus citations

Abstract

The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH₃NH₃PbI₃ onto a planar NiO layer and built a planar inverted ITO/NiO/CH₃NH₃PbI₃/PCBM/Al photovoltaic device. A device efficiency of 7.6% was achieved with an impressively high open-circuit voltage (V_oc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. (Graph Presented).

Original language	English
Pages (from-to)	547-553
Number of pages	7
Journal	ACS Photonics
Volume	1
Issue number	7
DOIs	https://doi.org/10.1021/ph5000067
State	Published - 16 Jul 2014
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2014 American Chemical Society.

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

NiO
perovskite
sequential deposition
solar cell

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Biotechnology
Atomic and Molecular Physics, and Optics
Electrical and Electronic Engineering

Access to Document

10.1021/ph5000067

Cite this

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title = "Sequential Deposition of CH3NH3PbI3 on Planar NiO Film for Efficient Planar Perovskite Solar Cells",

abstract = "The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16\%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH3NH3PbI3 onto a planar NiO layer and built a planar inverted ITO/NiO/CH3NH3PbI3/PCBM/Al photovoltaic device. A device efficiency of 7.6\% was achieved with an impressively high open-circuit voltage (Voc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. (Graph Presented).",

keywords = "NiO, perovskite, sequential deposition, solar cell",

author = "Long Hu and Jun Peng and Weiwei Wang and Zhe Xia and Jianyu Yuan and Jialing Lu and Xiaodong Huang and Wanli Ma and Huaibing Song and Wei Chen and Cheng, \{Yi Bing\} and Jiang Tang",

note = "Publisher Copyright: {\textcopyright} 2014 American Chemical Society.",

year = "2014",

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doi = "10.1021/ph5000067",

language = "English",

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T1 - Sequential Deposition of CH3NH3PbI3 on Planar NiO Film for Efficient Planar Perovskite Solar Cells

AU - Hu, Long

AU - Peng, Jun

AU - Wang, Weiwei

AU - Xia, Zhe

AU - Yuan, Jianyu

AU - Lu, Jialing

AU - Huang, Xiaodong

AU - Ma, Wanli

AU - Song, Huaibing

AU - Chen, Wei

AU - Cheng, Yi Bing

AU - Tang, Jiang

PY - 2014/7/16

Y1 - 2014/7/16

N2 - The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH3NH3PbI3 onto a planar NiO layer and built a planar inverted ITO/NiO/CH3NH3PbI3/PCBM/Al photovoltaic device. A device efficiency of 7.6% was achieved with an impressively high open-circuit voltage (Voc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. (Graph Presented).

AB - The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH3NH3PbI3 onto a planar NiO layer and built a planar inverted ITO/NiO/CH3NH3PbI3/PCBM/Al photovoltaic device. A device efficiency of 7.6% was achieved with an impressively high open-circuit voltage (Voc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. (Graph Presented).

KW - NiO

KW - perovskite

KW - sequential deposition

KW - solar cell

UR - https://www.scopus.com/pages/publications/84908021027

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DO - 10.1021/ph5000067

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ER -