Rate-based modelling of chilled ammonia process (cap) for co2 capture

Dawid P. Hanak; Chechet Biliyok; Hoi Yeung; Vasilije Manovic

doi:10.1016/B978-0-444-63456-6.50031-4

Rate-based modelling of chilled ammonia process (cap) for co₂ capture

Dawid P. Hanak^*, Chechet Biliyok, Hoi Yeung, Vasilije Manovic

^*Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceeding › Chapter › peer-review

Abstract

Chilled ammonia process (CAP) has been identified as a promising alternative to the monoethanolamine based capture process for post-combustion CO₂ capture. Therefore, a full-scale rate-based CAP capture plant model has been developed. First, the aqueous NH₃ process was modelled in Aspen Plus and validated with pilot-plant data. The model was modified to meet the CAP operating conditions, and then scaled-up to process the flue gas from 660 MW_el coal-fired power plant. The full-scale rate-based CAP model showed a substantial performance improvement through reducing the energy requirement for solvent regeneration by 27 % compared to the reference MEA process.

Original language	English
Title of host publication	Computer Aided Chemical Engineering
Publisher	Elsevier B.V.
Pages	181-186
Number of pages	6
DOIs	https://doi.org/10.1016/B978-0-444-63456-6.50031-4
State	Published - 2014
Externally published	Yes

Publication series

Name	Computer Aided Chemical Engineering
Volume	33
ISSN (Print)	1570-7946

Keywords

Carbon capture
Coal-fired power plant
Rate-based modelling chilled ammonia process

ASJC Scopus subject areas

General Chemical Engineering
Computer Science Applications

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1016/B978-0-444-63456-6.50031-4

Cite this

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title = "Rate-based modelling of chilled ammonia process (cap) for co2 capture",

abstract = "Chilled ammonia process (CAP) has been identified as a promising alternative to the monoethanolamine based capture process for post-combustion CO2 capture. Therefore, a full-scale rate-based CAP capture plant model has been developed. First, the aqueous NH3 process was modelled in Aspen Plus and validated with pilot-plant data. The model was modified to meet the CAP operating conditions, and then scaled-up to process the flue gas from 660 MWel coal-fired power plant. The full-scale rate-based CAP model showed a substantial performance improvement through reducing the energy requirement for solvent regeneration by 27 \% compared to the reference MEA process.",

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doi = "10.1016/B978-0-444-63456-6.50031-4",

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T1 - Rate-based modelling of chilled ammonia process (cap) for co2 capture

AU - Hanak, Dawid P.

AU - Biliyok, Chechet

AU - Yeung, Hoi

AU - Manovic, Vasilije

PY - 2014

Y1 - 2014

N2 - Chilled ammonia process (CAP) has been identified as a promising alternative to the monoethanolamine based capture process for post-combustion CO2 capture. Therefore, a full-scale rate-based CAP capture plant model has been developed. First, the aqueous NH3 process was modelled in Aspen Plus and validated with pilot-plant data. The model was modified to meet the CAP operating conditions, and then scaled-up to process the flue gas from 660 MWel coal-fired power plant. The full-scale rate-based CAP model showed a substantial performance improvement through reducing the energy requirement for solvent regeneration by 27 % compared to the reference MEA process.

AB - Chilled ammonia process (CAP) has been identified as a promising alternative to the monoethanolamine based capture process for post-combustion CO2 capture. Therefore, a full-scale rate-based CAP capture plant model has been developed. First, the aqueous NH3 process was modelled in Aspen Plus and validated with pilot-plant data. The model was modified to meet the CAP operating conditions, and then scaled-up to process the flue gas from 660 MWel coal-fired power plant. The full-scale rate-based CAP model showed a substantial performance improvement through reducing the energy requirement for solvent regeneration by 27 % compared to the reference MEA process.

KW - Carbon capture

KW - Coal-fired power plant

KW - Rate-based modelling chilled ammonia process

UR - https://www.scopus.com/pages/publications/84902988757

U2 - 10.1016/B978-0-444-63456-6.50031-4

DO - 10.1016/B978-0-444-63456-6.50031-4

M3 - Chapter

AN - SCOPUS:84902988757

T3 - Computer Aided Chemical Engineering

SP - 181

EP - 186

BT - Computer Aided Chemical Engineering

PB - Elsevier B.V.

ER -