Morphology and properties of waterborne polyurethane/CNT nanocomposite adhesives with various carboxyl acid salt groups

  • Mohammad Mizanur Rahman
  • , Eun Young Kim
  • , Kwon Taek Lim
  • , Won Ki Lee*
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

22 Scopus citations

Abstract

Three series of waterborne polyurethane (WBPU)/carbon nanotube (CNT) nanocomposites were prepared, and their morphology and properties with various 2,2-dimethylol propionic acid (DMPA) and CNT contents were investigated. The CNTs were homogeneously dispersed up to the optimum content in WBPU/CNT nanocomposite films. The degree of homogeneous CNT dispersion increased with increasing DMPA content in WBPU/CNT nanocomposite films. The optimum CNT content showed maximum tensile strength, Young's modulus and adhesive strength of WBPU/CNT nanocomposite film. The optimum CNT contents for WBPU/CNT nanocomposite samples containing 3.61, 5.16 and 5.86 wt% DMPA were about 0.50, 1.00 and 1.50 wt%, respectively. The WBPU/CNT nanocomposite adhesive showed higher adhesive strength at moderately high temperatures (40/60/80/100°C) compared to conventional WBPU. The highest adhesive strength at moderately high temperatures was found with 5.86 wt% DMPA and 1.5 wt% CNT content.

Original languageEnglish
Pages (from-to)839-850
Number of pages12
JournalJournal of Adhesion Science and Technology
Volume23
Issue number6
DOIs
StatePublished - 2009
Externally publishedYes

Bibliographical note

Funding Information:
This study was financially supported by the Pukyong National University in the 2008 Post-Doc. program and the Korea Science and Engineering Foundation (KOSEF) grant funded by the Korea government (MOST) (R01-2006-000-10042-0).

Keywords

  • Adhesives
  • CNT
  • Nanocomposites
  • Polyurethanes

ASJC Scopus subject areas

  • General Chemistry
  • Mechanics of Materials
  • Surfaces and Interfaces
  • Surfaces, Coatings and Films
  • Materials Chemistry

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