Melt miscibility and solid-state properties of metallocene LLDPE blends with HDPE: Influence of MM of LLDPE

Tayyab Hameed*, Ibnelwaleed A. Hussein

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

The influence of relative molecular mass (MM) of LLDPE on the rheological, thermal and mechanical properties of two sets of m-LLDPE/HDPE blends of low and high branch content (BC) was studied. Blends of m-LLDPE with linear HDPE reveal no influence of MM (60-100 kg/mol) on melt miscibility at low BC (about 20 branches/1 000 C). However, at high BC levels (about 40 branches/1 000 C), MM affects the melt miscibility of m-LLDPE/HDPE blends. The DSC results suggest that compatibility in the solid state is independent of MM and BC. For all blends studied, the HDPE-rich blends are found to contain single crystal populations, suggesting high degree of cocrystallization, whereas, m-LLDPE rich phase shows separate crystallization. Mechanical properties of these blends are found to be a strong function of blend compatibility and the specific properties of the blend components. In general, the high BC pairs show poor mechanical properties.

Original languageEnglish
Pages (from-to)183-187
Number of pages5
JournalJournal of Central South University of Technology (English Edition)
Volume14
Issue number1 SUPPL.
DOIs
StatePublished - Feb 2007

Bibliographical note

Funding Information:
The authors wish to acknowledge KFUPM for the financial support.

Keywords

  • Metallocene LLDPE
  • Miscibility
  • Molecular mass
  • Rheological property

ASJC Scopus subject areas

  • General Materials Science
  • Mechanics of Materials
  • Mechanical Engineering

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