Influence of short-chain branching of polyethylenes on the temperature dependence of rheological properties in shear

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75 Scopus citations

Abstract

This contribution describes the influence of short-chain branching on the temperature dependence of rheological properties of polyethylene (PE) melts in shear. The materials investigated are linear and short-chain branched, metallocene-catalyzed PEs of narrow molecular mass distribution. The linear visco-elastic properties are determined by dynamic-mechanical analysis. Short-chain branching (SCB) leads to an increase of the flow activation energy. The activation energy was found to increase linearly with rising weight comonomer content.

Original languageEnglish
Pages (from-to)2449-2454
Number of pages6
JournalMacromolecular Chemistry and Physics
Volume208
Issue number22
DOIs
StatePublished - 20 Nov 2007
Externally publishedYes

Keywords

  • Comonomer length and content
  • Flow activation energy
  • Polyethylenes
  • Rheology
  • Short-chain branching

ASJC Scopus subject areas

  • Condensed Matter Physics
  • Physical and Theoretical Chemistry
  • Organic Chemistry
  • Polymers and Plastics
  • Materials Chemistry

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