Floquet engineering of interlayer couplings: Tuning the magic angle of twisted bilayer graphene at the exit of a waveguide

We introduce an approach that allows one complete control over the modulation of the effective twist angle change in few-layer van der Waals heterostructures by irradiating them with longitudinal waves of light at the end of a waveguide. As a specific application, we consider twisted bilayer graphene and show that one can tune the magic angles to be either larger or smaller, allowing in situ experimental control of the phase diagram of this and other related materials. A waveguide allows one to circumvent the free-space constraints on the absence of longitudinal electric field components of light. We propose to place twisted bilayer graphene at a specific location at the exit of a waveguide, such that it is subjected to purely longitudinal components of a transverse magnetic mode wave.