Exponential decay in a spin bath

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69 Scopus citations

Abstract

We show that the coherence of an electron spin interacting with a bath of nuclear spins can exhibit a well-defined purely exponential decay for special ("narrowed") bath initial conditions in the presence of a strong applied magnetic field. This is in contrast to the typical case, where spin-bath dynamics have been investigated in the non-Markovian limit, giving superexponential or power-law decay of correlation functions. We calculate the relevant decoherence time T2 explicitly for free-induction decay and find a simple expression with dependence on bath polarization, magnetic field, shape of the electron wave function, dimensionality, total nuclear spin I, and isotopic concentration for experimentally relevant heteronuclear-spin systems.

Original languageEnglish
Article number125329
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume77
Issue number12
DOIs
StatePublished - 20 Mar 2008
Externally publishedYes

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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