Energy storage and piezoelectric properties of lead‐free SrTiO3-modified 0.965Bi0.5Na0.5TiO3–0.035BaTiO3 ceramics

Muhammad Munir; Muhammad Habib; Salman Ali Khan; Myong Ho Kim; Soonil Lee; Tae Kwon Song; Abrar H. Baluch; Ayse Turak; Ali Hussain

doi:10.1007/s10854-021-05728-6

Energy storage and piezoelectric properties of lead‐free SrTiO₃-modified 0.965Bi_0.5Na_0.5TiO₃–0.035BaTiO₃ ceramics

Muhammad Munir
, Muhammad Habib
, Salman Ali Khan
, Myong Ho Kim
, Soonil Lee
, Tae Kwon Song
, Abrar H. Baluch
, Ayse Turak^*
, Ali Hussain^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

11 Scopus citations

Abstract

This manuscript reports the synthesis and piezoelectric properties of strontium titanate, SrTiO₃-modified bismuth sodium titanate-barium titanate, 0.965Bi_0.5Na_0.5TiO₃–0.035BaTiO_3, (BNBT-xST, x = 0.00−0.30) ceramics produced by facile low temperature sol–gel and hydrothermal methods. Close inspection of the X-ray diffraction profile through Rietveld refinement indicates ST modification in BNBT leads to a phase transition from the dominant rhombohedral phase to a single tetragonal phase. This structural transition leads to enhancement of electromechanical and energy storage properties. A large dynamic piezoelectric coefficient (d^*₃₃ = 350 pC/V) was observed for BNBT-0.1ST sample. High energy storage density (W_rec = 0.37) and large energy storage efficiency (η = 75%) were observed at 75 °C for the BNBT-0.3ST sample. The energy storage response of the tunable ferrorelectric ceramics suggests their possible use for high-performance dielectric capacitor applications.

Original language	English
Pages (from-to)	10712-10725
Number of pages	14
Journal	Journal of Materials Science: Materials in Electronics
Volume	32
Issue number	8
DOIs	https://doi.org/10.1007/s10854-021-05728-6
State	Published - Apr 2021
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2021, The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature.

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Atomic and Molecular Physics, and Optics
Condensed Matter Physics
Electrical and Electronic Engineering

Access to Document

10.1007/s10854-021-05728-6

Cite this

@article{83093e483d394af58e3429613eb6aade,

title = "Energy storage and piezoelectric properties of lead‐free SrTiO3-modified 0.965Bi0.5Na0.5TiO3–0.035BaTiO3 ceramics",

abstract = "This manuscript reports the synthesis and piezoelectric properties of strontium titanate, SrTiO3-modified bismuth sodium titanate-barium titanate, 0.965Bi0.5Na0.5TiO3–0.035BaTiO3, (BNBT-xST, x = 0.00−0.30) ceramics produced by facile low temperature sol–gel and hydrothermal methods. Close inspection of the X-ray diffraction profile through Rietveld refinement indicates ST modification in BNBT leads to a phase transition from the dominant rhombohedral phase to a single tetragonal phase. This structural transition leads to enhancement of electromechanical and energy storage properties. A large dynamic piezoelectric coefficient (d*33 = 350 pC/V) was observed for BNBT-0.1ST sample. High energy storage density (Wrec = 0.37) and large energy storage efficiency (η = 75\%) were observed at 75 °C for the BNBT-0.3ST sample. The energy storage response of the tunable ferrorelectric ceramics suggests their possible use for high-performance dielectric capacitor applications.",

author = "Muhammad Munir and Muhammad Habib and Khan, \{Salman Ali\} and Kim, \{Myong Ho\} and Soonil Lee and Song, \{Tae Kwon\} and Baluch, \{Abrar H.\} and Ayse Turak and Ali Hussain",

note = "Publisher Copyright: {\textcopyright} 2021, The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature.",

year = "2021",

month = apr,

doi = "10.1007/s10854-021-05728-6",

language = "English",

volume = "32",

pages = "10712--10725",

journal = "Journal of Materials Science: Materials in Electronics",

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AU - Munir, Muhammad

AU - Habib, Muhammad

AU - Khan, Salman Ali

AU - Kim, Myong Ho

AU - Lee, Soonil

AU - Song, Tae Kwon

AU - Baluch, Abrar H.

AU - Turak, Ayse

AU - Hussain, Ali

PY - 2021/4

Y1 - 2021/4

N2 - This manuscript reports the synthesis and piezoelectric properties of strontium titanate, SrTiO3-modified bismuth sodium titanate-barium titanate, 0.965Bi0.5Na0.5TiO3–0.035BaTiO3, (BNBT-xST, x = 0.00−0.30) ceramics produced by facile low temperature sol–gel and hydrothermal methods. Close inspection of the X-ray diffraction profile through Rietveld refinement indicates ST modification in BNBT leads to a phase transition from the dominant rhombohedral phase to a single tetragonal phase. This structural transition leads to enhancement of electromechanical and energy storage properties. A large dynamic piezoelectric coefficient (d*33 = 350 pC/V) was observed for BNBT-0.1ST sample. High energy storage density (Wrec = 0.37) and large energy storage efficiency (η = 75%) were observed at 75 °C for the BNBT-0.3ST sample. The energy storage response of the tunable ferrorelectric ceramics suggests their possible use for high-performance dielectric capacitor applications.

AB - This manuscript reports the synthesis and piezoelectric properties of strontium titanate, SrTiO3-modified bismuth sodium titanate-barium titanate, 0.965Bi0.5Na0.5TiO3–0.035BaTiO3, (BNBT-xST, x = 0.00−0.30) ceramics produced by facile low temperature sol–gel and hydrothermal methods. Close inspection of the X-ray diffraction profile through Rietveld refinement indicates ST modification in BNBT leads to a phase transition from the dominant rhombohedral phase to a single tetragonal phase. This structural transition leads to enhancement of electromechanical and energy storage properties. A large dynamic piezoelectric coefficient (d*33 = 350 pC/V) was observed for BNBT-0.1ST sample. High energy storage density (Wrec = 0.37) and large energy storage efficiency (η = 75%) were observed at 75 °C for the BNBT-0.3ST sample. The energy storage response of the tunable ferrorelectric ceramics suggests their possible use for high-performance dielectric capacitor applications.

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