Skip to main navigation Skip to search Skip to main content

Dark states enhance the photocell power via phononic dissipation

  • Yiteng Zhang
  • , Aaron Wirthwein
  • , Fahhad H. Alharbi
  • , Gregory S. Engel
  • , Sabre Kais*
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

17 Scopus citations

Abstract

The high efficiency of the photon-to-charge conversion process found in photosynthetic complexes has inspired researchers to explore a new route for designing artificial photovoltaic materials. Quantum coherence can provide a mean to surpass the Shockley-Quiesser device concept limit by reducing the radiative recombination. Taking inspiration from these new discoveries, we consider a linearly-aligned system as a light-harvesting antennae composed of two-level optical emitters coupled with each other by dipole-dipole interactions. Our simulations show that the certain dark states can enhance the power with the aid of intra-band phononic dissipation. Due to cooperative effects, the output power will be improved when incorporating more emitters in the linear system.

Original languageEnglish
Pages (from-to)31845-31849
Number of pages5
JournalPhysical Chemistry Chemical Physics
Volume18
Issue number46
DOIs
StatePublished - 2016
Externally publishedYes

Bibliographical note

Publisher Copyright:
© the Owner Societies 2016.

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 7 - Affordable and Clean Energy
    SDG 7 Affordable and Clean Energy

ASJC Scopus subject areas

  • General Physics and Astronomy
  • Physical and Theoretical Chemistry

Fingerprint

Dive into the research topics of 'Dark states enhance the photocell power via phononic dissipation'. Together they form a unique fingerprint.

Cite this